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Abstract: We applied the hard and soft acid-base (HSAB) model (Xu and Harsh 1990a, 1990b) to bivalent cation exchange on a purified Ca-montmorillonite. As a result, a satisfactory model is proposed to...
Abstract: A theoretical model describing the interaction between crystalline swelling and cation exchange selectivity is proposed for expanding 2:1 phyllosilicates. The model is based on the assumptio...
A critical demand in environmental modeling and a desirable but elusive goal of research on the ion exchange properties of the charged solid surface has been to determine the selectivity coefficient f...
A critical demand in environmental modeling and a desirable but elusive goal of research on the ion exchange properties of the charged solid surface has been to determine the selectivity coefficient f...
Ion-exchange experiments in expanding clay minerals conducted over a wide range of surface ionic compositions and ionic strength produce variable mass-action selectivity coefficients. When the exchang...
Two variables must be considered when calculating exchange free energies (ΔG0ex) for 2:1 clays: (1) anionic field strength, as expressed by equivalent anionic radius (ra), and (2) interlayer water con...
The decreasing preference of montmorillonite for K+ relative to Na+ as the clay adsorbs increasing amounts of K+ is shown to be the general rule for the exchange of strongly hydrating ions by weakly h...
Smectite (from South Dakota, Wyoming, and Mississippi) and vermiculite (Transvaal) were treated with solutions of Al(OH)B(3−B)+, with B varying from 0 to 2.5. The average basicity (OH/Al = B) of...
Abstract: Clay materials separated from estuarine sediments in Louisiana exhibit a selectivity for exchangeable calcium in laboratory experiments. The studies were conducted at 25°C and 60°C in mixed ...
Abstract: The Ca-K exchange isotherms were determined at two temperatures for two highly montmorillonitic iron-rich soil clays in their oxidized and reduced states. The thermodynamic parameters K, ΔG0...
The use of electron diffraction contrast to detect local concentrations of interlayer cations in mica-vermiculites was examined. Cs and Mg, because of their contrasting atomic scattering amplitudes fo...
The adsorption of hydroxy-Al by the 2?? ?size fractions of muscovite, biotite, K-depleted micas, vermiculite and montmorillonite was studied. The differences in the amounts of hydroxy-Al adsorbed were...
Abstract: Selectivity of a number of vermiculites, montmorillonites and micas for K and Cs ions was determined by sorption of these ions from equilibrium solutions of diverse concentrations. The selec...

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