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Many mixed-valence systems involve two or more states with different electric dipole moments whose magnitudes depend upon the charge transfer distance and the degree of delocalization; these systems c...
The electronic structure of the binuclear copper complex [Cu(2)(L)](3+) [L = N(CH(2)CH(2)N(H)CH(2)CH(2)N(H)CH(2)CH(2))(3)N] has been investigated by resonance Raman and electroabsorption spectroscopy....
Stark (electroabsorption) spectroscopy can provide quantitative information on the change in dipole moment and polarizability for an electronic transition. In the case of mixed-valence transitions, th...
Many experimental and theoretical approaches have been developed to characterize the chemical and physical properties of mixed-valence complexes. These molecules may possess metals in differing oxidat...
The electron transfer kinetics of mixed-valence systems is studied via solving the eigenstructure of the twostate nonadiabatic diffusion operator for a wide range of electronic coupling constants and ...
An adiabatic picture is proposed to analyze short-time electronic coherence and dephasing in mixed-valence systems,which cannot be described by the Redfield equation or the golden-rule rate theory. In...

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